Five portable Bruker EM27/SUN FTIR spectrometers have been used for the accurate and precise observation of column averaged abundances of CO2 and CH4 around the megacity Berlin. In the first part of this work (Frey et al., 2015) we have presented the various measures that were undertaken to ensure that the observations are consistent between sites, accurate and precise. Here, we present the recorded time series of XCH4 and XCO2 and demonstrate that the CO2 emissions of Berlin can be clearly identified in the observations. A simple dispersion model is applied which indicates a total strength of the Berlin source of about 0.8 t CO2 s-1. In the Supplement of this work, we provide the measured dataset and auxiliary data. We hope that the model community will exploit this unique dataset for state-of-the art inversion studies of CO2 and CH4 sources in the Berlin area.