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Partitioning and budget of inorganic and organic chlorine species observed by MIPAS-B and TELIS in the Arctic in March 2011

Wetzel, G.; Oelhaf, H.; Birk, M.; de Lange, A.; Engel, A.; Friedl-Vallon, F.; Kirner, O.; Kleinert, A.; Maucher, G.; Nordmeyer, H.; Orphal, J.; Ruhnke, R.; Sinnhuber, B.-M.; Vogt, P.

Abstract (englisch):
The Arctic winter 2010/2011 was characterized by a persistent vortex with extremely low temperatures in the lower stratosphere above northern Scandinavia leading to a strong activation of chlorine compounds (ClOx) like Cl, Cl2, ClO, ClOOCl, OClO, and HOCl, which rapidly destroyed ozone when sunlight returned after winter solstice. The MIPAS-B (Michelson Interferometer for Passive Atmospheric Sounding) and TELIS (TErahertz and submillimeter LImb Sounder) balloon measurements obtained in northern Sweden on 31 March 2011 inside the polar vortex have provided vertical profiles of inorganic and organic chlorine species as well as diurnal variations of ClO around sunrise over the whole altitude range in which chlorine has been undergoing activation and deactivation. This flight was performed at the end of the winter during the last phase of ClOx deactivation. The complete inorganic and organic chlorine partitioning and budget for 31 March 2011, assumed to be representative for the late-winter Arctic stratosphere, has been derived by combining MIPAS-B and TELIS simultaneously observed molecules. A total chlorine amount of 3.41 ± 0.30 parts per billion by volume is inferred from the measurements (above 24 km). ... mehr

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Volltext §
DOI: 10.5445/IR/1000051428
Originalveröffentlichung
DOI: 10.5194/acp-15-8065-2015
Scopus
Zitationen: 9
Web of Science
Zitationen: 9
Coverbild
Zugehörige Institution(en) am KIT Fakultät für Physik (PHYSIK)
Steinbuch Centre for Computing (SCC)
Institut für Meteorologie und Klimaforschung - Atmosphärische Spurenstoffe und Fernerkundung (IMK-ASF)
Publikationstyp Zeitschriftenaufsatz
Jahr 2015
Sprache Englisch
Identifikator ISSN: 1680-7316, 1680-7324
urn:nbn:de:swb:90-514280
KITopen-ID: 1000051428
HGF-Programm 12.04 (POF III, LK 01)
Erschienen in Atmospheric chemistry and physics
Band 15
Heft 14
Seiten 8065-8076
Bemerkung zur Veröffentlichung Gefördert durch den KIT-Publikationsfonds
Nachgewiesen in Web of Science
Scopus
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