Simulation-Assisted Design of Polycrystalline Zeolite Catalysts
Abstract (englisch):
A crystallite-pore network model (CPNM) was developed to simulate diffusion and reaction in polycrystalline zeolite catalysts. It has been applied to simulate the direct DME synthesis in bifunctional core-shell catalyst with an H-ZSM-5 shell, and xylene isomerization in an H-ZSM-5 membrane. The structural effects of H-ZSM-5 catalysts on these two reaction systems were studied via simulations. Some guidances on the catalyst optimization were also given from the simulation results.
| Zugehörige Institution(en) am KIT | Institut für Mikroverfahrenstechnik (IMVT) |
| Publikationstyp | Hochschulschrift |
| Publikationsjahr | 2016 |
| Sprache | Englisch |
| Identifikator | urn:nbn:de:swb:90-544145 KITopen-ID: 1000054414 |
| HGF-Programm | 37.03.02 (POF III, LK 01) Components and Process Development |
| Verlag | Karlsruher Institut für Technologie (KIT) |
| Art der Arbeit | Dissertation |
| Prüfungsdaten | 14.04.2016 |
| Schlagwörter | crystallite-pore network model, surface diffusion, microporous materials, modeling of porous catalysts |
| Relationen in KITopen |