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Evaluation of European air quality modelled by CAMx including the volatility basis set scheme

Ciarelli, Giancarlo; Aksoyoglu, Sebnem; Crippa, Monica; Jimenez, Jose-Luis; Nemitz, Eriko; Sellegri, Karine; Aijala, Mikko; Carbone, Samara; Mohr, Claudia; O'Dowd, Colin; Poulain, Laurent; Baltensperger, Urs; Prevot, Andre S.H.

Abstract:
Four periods of EMEP (European Monitoring and Evaluation Programme) intensive measurement campaigns (June 2006, January 2007, September–October 2008 and February–March 2009) were modelled using the regional air quality model CAMx with VBS (volatility basis set) approach for the first time in Europe within the framework of the EURODELTA-III model intercomparison exercise. More detailed analysis and sensitivity tests were performed for the period of February–March 2009 and June 2006 to investigate the uncertainties in emissions as well as to improve the modelling of organic aerosol (OA). Model performance for selected gas phase species and PM$_{2.5}$ was evaluated using the European air quality database AirBase. Sulfur dioxide (SO$_{2}$) and ozone (O$_{3}$) were found to be overestimated for all the four periods, with O3 having the largest mean bias during June 2006 and January–February 2007 periods (8.9 pbb and 12.3 ppb mean biases respectively). In contrast, nitrogen dioxide (NO$_{2}$) and carbon monoxide (CO) were found to be underestimated for all the four periods. CAMx reproduced both total concentrations and monthly variations o ... mehr


Zugehörige Institution(en) am KIT Institut für Meteorologie und Klimaforschung - Atmosphärische Aerosolforschung (IMK-AAF)
Publikationstyp Zeitschriftenaufsatz
Jahr 2016
Sprache Englisch
Identifikator DOI: 10.5194/acp-16-10313-2016
ISSN: 1680-7316, 1680-7324
URN: urn:nbn:de:swb:90-601037
KITopen ID: 1000060103
HGF-Programm 12.03.03; LK 01
Erschienen in Atmospheric chemistry and physics
Band 16
Heft 16
Seiten 10313-10332
Lizenz CC BY 3.0 DE: Creative Commons Namensnennung 3.0 Deutschland
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