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An emission module for ICON-ART 2.0: implementation and simulations of acetone

Weimer, Michael; Schröter, Jennifer; Eckstein, Johannes; Deetz, Konrad; Neumaier, Marco; Fischbeck, Garlich; Hu, Lu; Millet, Dylan B.; Rieger, Daniel; Vogel, Heike; Vogel, Bernhard; Reddmann, Thomas; Kirner, Oliver; Ruhnke, Roland; Braesicke, Peter

Abstract:
We present a recently developed emission module for the ICON (ICOsahedral Non-hydrostatic)-ART (Aerosols and Reactive Trace gases) modelling framework. The emission module processes external flux data sets and increments the tracer volume mixing ratios in the boundary layer accordingly.

The performance of the emission module is illustrated with simulations of acetone, using a simplified chemical depletion mechanism based on a reaction with OH and photolysis only. In our model setup, we calculate a tropospheric acetone lifetime of 33 days, which is in good agreement with the literature. We compare our results with ground-based as well as with airborne IAGOS-CARIBIC measurements in the upper troposphere and lowermost stratosphere (UTLS) in terms of phase and amplitude of the annual cycle. In all our ICON-ART simulations the general seasonal variability is well represented but uncertainties remain concerning the magnitude of the acetone mixing ratio in the UTLS region.

In addition, the module for online calculations of biogenic emissions (MEGAN2.1) is implemented in ICON-ART and can replace the offline biogenic emission data sets. ... mehr

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Volltext §
DOI: 10.5445/IR/1000071383
Originalveröffentlichung
DOI: 10.5194/gmd-10-2471-2017
Scopus
Zitationen: 3
Web of Science
Zitationen: 3
Coverbild
Zugehörige Institution(en) am KIT Fakultät für Physik (PHYSIK)
Steinbuch Centre for Computing (SCC)
Institut für Meteorologie und Klimaforschung - Atmosphärische Spurenstoffe und Fernerkundung (IMK-ASF)
Institut für Meteorologie und Klimaforschung - Forschungsbereich Troposphäre (IMK-TRO)
Publikationstyp Zeitschriftenaufsatz
Jahr 2017
Sprache Englisch
Identifikator ISSN: 1991-9603, 1991-959X
urn:nbn:de:swb:90-713833
KITopen-ID: 1000071383
HGF-Programm 12.03.04 (POF III, LK 01)
Erschienen in Geoscientific model development
Band 10
Heft 6
Seiten 2471–2494
Bemerkung zur Veröffentlichung Gefördert durch den KIT-Publikationsfonds
Nachgewiesen in Web of Science
Scopus
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