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URN: urn:nbn:de:swb:90-730265

A comparison of two chemistry and aerosol schemes on the regional scale and the resulting impact on radiative properties and liquid- and ice-phase aerosol-cloud interactions

Glassmeier, Franziska; Possner, Anna; Vogel, Bernhard; Vogel, Heike; Lohmann, Ulrike

Abstract:
The complexity of atmospheric aerosol causes large uncertainties in its parameterization in atmospheric models. In a process-based comparison of two aerosol and chemistry schemes within the regional atmospheric modeling framework COSMO-ART (Consortium for Small-Scale Modelling, Aersosol and Reactive Trace gases extension), we identify key sensitivities of aerosol parameterizations. We consider the aerosol module MADE (Modal Aerosol Dynamics model for Europe) in combination with full gas-phase chemistry and the aerosol module M7 in combination with a constant-oxidant-field-based sulfur cycle. For a Saharan dust outbreak reaching Europe, modeled aerosol populations are more sensitive to structural differences between the schemes, in particular the consideration of aqueous-phase sulfate production, the selection of aerosol species and modes, and modal composition, than to parametric choices like modal standard deviation and the parameterization of aerosol dynamics. The same observation applies to aerosol optical depth (AOD) and the concentrations of cloud condensation nuclei (CCN). Differences in the concentrations of ice-nucleating pa ... mehr


Zugehörige Institution(en) am KIT Institut für Meteorologie und Klimaforschung - Forschungsbereich Troposphäre (IMK-TRO)
Publikationstyp Zeitschriftenaufsatz
Jahr 2017
Sprache Englisch
Identifikator ISSN: 1680-7316, 1680-7324
URN: urn:nbn:de:swb:90-730265
KITopen ID: 1000073026
Erschienen in Atmospheric chemistry and physics
Band 17
Heft 14
Seiten 8651-8680
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