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Verlagsausgabe
DOI: 10.5445/IR/1000082988
Veröffentlicht am 22.05.2018
Originalveröffentlichung
DOI: 10.5194/acp-18-2883-2018
Scopus
Zitationen: 8
Web of Science
Zitationen: 7

α-Pinene secondary organic aerosol at low temperature: chemical composition and implications for particle viscosity

Huang, Wei; Saathoff, Harald; Pajunoja, Aki; Shen, Xiaoli; Naumann, Karl-Heinz; Wagner, Robert; Virtanen, Annele; Leisner, Thomas; Mohr, Claudia

Abstract:
Chemical composition, size distributions, and degree of oligomerization of secondary organic aerosol (SOA) from α-pinene (C10H16) ozonolysis were investigated for low-temperature conditions (223 K). Two types of experiments were performed using two simulation chambers at the Karlsruhe Institute of Technology: the Aerosol Preparation and Characterization (APC) chamber, and the Aerosol Interaction and Dynamics in the Atmosphere (AIDA) chamber. Experiment type 1 simulated SOA formation at upper tropospheric conditions: SOA was generated in the AIDA chamber directly at 223 K at 61 % relative humidity (RH; experiment termed “cold humid”, CH) and for comparison at 6 % RH (experiment termed “cold dry”, CD) conditions. Experiment type 2 simulated SOA uplifting: SOA was formed in the APC chamber at room temperature (296 K) and < 1 % RH (experiment termed “warm dry”, WD) or 21 % RH (experiment termed “warm humid”, WH) conditions, and then partially transferred to the AIDA chamber kept at 223 K, and 61 % RH (WDtoCH) or 30 % RH (WHtoCH), respectively. Precursor concentrations varied between 0.7 and 2.2 ppm α-pinene, and between 2.3 and 1.8 p ... mehr


Zugehörige Institution(en) am KIT Institut für Geographie und Geoökologie (IFGG)
Institut für Meteorologie und Klimaforschung - Atmosphärische Aerosolforschung (IMK-AAF)
Publikationstyp Zeitschriftenaufsatz
Jahr 2018
Sprache Englisch
Identifikator ISSN: 1680-7324
URN: urn:nbn:de:swb:90-829884
KITopen-ID: 1000082988
HGF-Programm 12.03.03 (POF III, LK 01)
Erschienen in Atmospheric chemistry and physics
Band 18
Heft 4
Seiten 2883–2898
Bemerkung zur Veröffentlichung Gefördert durch den KIT-Publikationsfonds
Vorab online veröffentlicht am 28.02.2018
Nachgewiesen in Web of Science
Scopus
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