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Moving Frontiers in Transition Metal Catalysis: Synthesis, Characterization and Modeling

Sharapa, D. I. ORCID iD icon 1; Doronkin, D. E. ORCID iD icon 1,2; Studt, F. 1,2; Grunwaldt, J.-D. ORCID iD icon 1,2; Behrens, S. 1
1 Institut für Katalyseforschung und -technologie (IKFT), Karlsruher Institut für Technologie (KIT)
2 Institut für Technische Chemie und Polymerchemie (ITCP), Karlsruher Institut für Technologie (KIT)


Nanosized transition metal particles are important materials in catalysis with a key role not only in academic research but also in many processes with industrial and societal relevance. Although small improvements in catalytic properties can lead to significant economic and environmental impacts, it is only now that knowledge-based design of such materials is emerging, partly because the understanding of catalytic mechanisms on nanoparticle surfaces is increasingly improving. A knowledge-based design requires bottom-up synthesis of well-defined model catalysts, an understanding of the catalytic nanomaterials “at work” (operando), and both a detailed understanding and a prediction by theoretical methods. This article reports on progress in colloidal synthesis of transition metal nanoparticles for preparation of model catalysts to close the materials gap between the discoveries of fundamental surface science and industrial application. The transition metal particles, however, often undergo extensive transformations when applied to the catalytic process and much progress has recently been achieved operando characterization techniques under relevant reaction conditions. ... mehr

Verlagsausgabe §
DOI: 10.5445/IR/1000092875
Veröffentlicht am 10.04.2019
DOI: 10.1002/adma.201807381
Zitationen: 37
Web of Science
Zitationen: 38
Zitationen: 38
Cover der Publikation
Zugehörige Institution(en) am KIT Institut für Katalyseforschung und -technologie (IKFT)
Institut für Technische Chemie und Polymerchemie (ITCP)
Publikationstyp Zeitschriftenaufsatz
Publikationsdatum 27.06.2019
Sprache Englisch
Identifikator ISSN: 0935-9648, 1521-4095
KITopen-ID: 1000092875
HGF-Programm 43.22.02 (POF III, LK 01) Nanocatalysis
Weitere HGF-Programme 56.98.01 (POF III, LK 01) Betrieb in MML
Erschienen in Advanced materials
Verlag John Wiley and Sons
Band 31
Heft 26
Seiten Art.Nr. 1807381
Vorab online veröffentlicht am 25.02.2019
Nachgewiesen in Web of Science
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