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Mesoporous H‐ZSM‐5 for the Conversion of Dimethyl Ether to Hydrocarbons

Zimmermann, Michael C.; Otto, Thomas N.; Wodarz, Simon; Zevaco, Thomas A.; Pitter, Stephan

Abstract:
The potential of hierarchical H‐ZSM‐5 zeolites was studied for the conversion of DME to fuel‐compatible hydrocarbons. For this purpose, hierarchical H‐ZSM‐5 zeolites have been prepared from commercial H‐ZSM‐5 by desilication and organosilane‐directed hydrothermal synthesis. The zeolites were characterized by X‐ray diffraction, NH3‐TPD, DRIFTS, and N2 physisorption measurements. The catalysts have been tested in a tube reactor (1 bar, 648 K). The results indicate important structural changes in framework and acidic sites, which are significant for the synthesis of gasoline‐range hydrocarbons.

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Verlagsausgabe §
DOI: 10.5445/IR/1000104129
Veröffentlicht am 12.12.2019
Originalveröffentlichung
DOI: 10.1002/cite.201800217
Scopus
Zitationen: 2
Web of Science
Zitationen: 2
Cover der Publikation
Zugehörige Institution(en) am KIT Institut für Katalyseforschung und -Technologie (IKFT)
Publikationstyp Zeitschriftenaufsatz
Publikationsmonat/-jahr 09.2019
Sprache Deutsch
Identifikator ISSN: 0009-286X, 1522-2640
KITopen-ID: 1000104129
HGF-Programm 37.03.02 (POF III, LK 01)
Components and Process Development
Erschienen in Chemie - Ingenieur - Technik
Band 91
Heft 9
Seiten 1302–1313
Vorab online veröffentlicht am 07.08.2019
Nachgewiesen in Scopus
Web of Science
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