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Production of CO₂-neutral liquid fuels by integrating Fischer-Tropsch synthesis and hydrocracking in a single micro-structured reactor: Performance evaluation of different configurations by factorial design experiments

Kirsch, Hannah; Lochmahr, Natalie; Staudt, Christiane; Pfeifer, Peter; Dittmeyer, Roland

Abstract:
Humankind must drastically reduce CO$_{2}$ emissions within the next three decades to limit global climate change. Defossilization of the transport sector must contribute to the achievement of this ambitious aim. One promising option is the production of synthetic liquid fuels from CO$_{2}$, water, and renewable electrical energy. Liquid fuels will also be used in the future, especially for heavy-duty vehicles and aviation. We studied the production of liquid fuels by integration of Fischer-Tropsch Synthesis (FTS) and Hydrocracking (HC) in a single micro-structured reactor. Thereby, we addressed the aspects of process simplification and process intensification. Both are particularly important for flexible small-scale plants for decentralized application in context of the energy transition. In this study, we systematically investigated the performance of the integrated FTS/HC process depending on different operating conditions (pressure, temperature, weight hourly space velocity, H$_{2}$/CO synthesis gas ratio) and integration configurations by applying a factorial design approach. Beyond the selectivity of the process towards liquid fuels, we especially focus on the product quality affected by the type of produced hydrocarbons. ... mehr

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Verlagsausgabe §
DOI: 10.5445/IR/1000120160
Veröffentlicht am 03.07.2020
Originalveröffentlichung
DOI: 10.1016/j.cej.2020.124553
Scopus
Zitationen: 3
Web of Science
Zitationen: 2
Dimensions
Zitationen: 4
Cover der Publikation
Zugehörige Institution(en) am KIT Institut für Mikroverfahrenstechnik (IMVT)
Publikationstyp Zeitschriftenaufsatz
Publikationsdatum 01.08.2020
Sprache Englisch
Identifikator ISSN: 1385-8947
KITopen-ID: 1000120160
HGF-Programm 37.03.02 (POF III, LK 01) Components and Process Development
Erschienen in The chemical engineering journal
Verlag Elsevier
Band 393
Seiten Art. Nr.: 124553
Schlagwörter Fischer-Tropsch synthesis, Hydrocracking, Power-to-Liquid, Synthetic fuels, Process integration, Micro-structured reactor
Nachgewiesen in Dimensions
Web of Science
Scopus
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