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A convolution of observational and model data to estimate age of air spectra in the northern hemispheric lower stratosphere

Hauck, M.; Bönisch, H.; Hoor, P.; Keber, T.; Ploeger, F.; Schuck, T. J.; Engel, A.

Derivation of mean age of air (AoA) and age spectra from atmospheric measurements remains a challenge and often requires output from atmospheric models. This study tries to minimize the direct influence of model output and presents an extension and application of a previously established inversion method to derive age spectra from mixing ratios of long- and short-lived trace gases. For a precise description of cross-tropopause transport processes, the inverse method is extended to incorporate air entrainment into the stratosphere across the tropical and extratropical tropopause. We first use simulations with the Chemical Lagrangian Model of the Stratosphere (CLaMS) to provide a general proof of concept of the extended principle in a controllable and consistent environment, where the method is applied to an idealized set of 10 trace gases with predefined constant lifetimes and compared to reference model age spectra. In the second part of the study we apply the extended inverse method to atmospheric measurements of multiple long- and short-lived trace gases measured aboard the High Altitude and Long Range (HALO) research aircraft during the two research campaigns POLSTRACC–GW-LCYCLE–SALSA (PGS) and Wave-driven Isentropic Exchange (WISE). ... mehr

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Verlagsausgabe §
DOI: 10.5445/IR/1000123391
Veröffentlicht am 09.09.2020
DOI: 10.5194/acp-20-8763-2020
Zitationen: 4
Web of Science
Zitationen: 4
Zitationen: 4
Cover der Publikation
Zugehörige Institution(en) am KIT Institut für Meteorologie und Klimaforschung - Atmosphärische Spurenstoffe und Fernerkundung (IMK-ASF)
KIT-Zentrum Klima und Umwelt (ZKU)
Publikationstyp Zeitschriftenaufsatz
Publikationsdatum 24.07.2020
Sprache Englisch
Identifikator ISSN: 1680-7316, 1680-7324
KITopen-ID: 1000123391
Erschienen in Atmospheric chemistry and physics
Verlag European Geosciences Union (EGU)
Band 20
Heft 14
Seiten 8763-8785
Nachgewiesen in Web of Science
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