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HIPPIE: a new platform for ambient-pressure X-ray photoelectron spectroscopy at the MAX IV Laboratory

Zhu, S.; Scardamaglia, M.; Kundsen, J.; Sankari, R.; Tarawneh, H.; Temperton, R.; Pickworth, L.; Cavalca, F.; Wang, C.; Tissot, H.; Weissenrieder, J.; Hagman, B.; Gustafson, J.; Kaya, S.; Lindgren, F.; Källquist, I.; Maibach, J. 1; Hahlin, M.; Boix, V.; ... mehr

HIPPIE is a soft X-ray beamline on the 3 GeV electron storage ring of the MAX IV Laboratory, equipped with a novel ambient-pressure X-ray photoelectron spectroscopy (APXPS) instrument. The endstation is dedicated to performing in situ and operando X-ray photoelectron spectroscopy experiments in the presence of a controlled gaseous atmosphere at pressures up to 30 mbar [1 mbar = 100 Pa] as well as under ultra-high vacuum conditions. The photon energy range is 250 to 2200 eV in planar polarization and with photon fluxes >10$^{12}$ photons s$^{-1}$ (500 mA ring current) at a resolving power of greater than
10000 and up to a maximum of 32000. The endstation currently provides two sample environments: a catalysis cell and an electrochemical/liquid cell. The former allows APXPS measurements of solid samples in the presence of a gaseous atmosphere (with a mixture of up to eight gases and a vapour of a liquid) and simultaneous analysis of the inlet/outlet gas composition by online mass spectrometry. The latter is a more versatile setup primarily designed for APXPS at the solid–liquid (dip-and-pull setup) or liquid–gas (liquid microjet) interfaces under full electrochemical control, and it can also be used as an open port for ad hoc-designed non-standard APXPS experiments with different sample environments. ... mehr

Verlagsausgabe §
DOI: 10.5445/IR/1000130913
Veröffentlicht am 31.03.2021
DOI: 10.1107/S160057752100103X
Zitationen: 21
Web of Science
Zitationen: 12
Zitationen: 17
Cover der Publikation
Zugehörige Institution(en) am KIT Institut für Angewandte Materialien – Energiespeichersysteme (IAM-ESS)
Publikationstyp Zeitschriftenaufsatz
Publikationsjahr 2021
Sprache Englisch
Identifikator ISSN: 1600-5775, 0909-0495
KITopen-ID: 1000130913
HGF-Programm 38.02.01 (POF IV, LK 01) Fundamentals and Materials
Erschienen in Journal of synchrotron radiation
Verlag International Union of Crystallography
Band 28
Seiten 624-636
Schlagwörter APXPS, operando, in situ, synchrotron, catalysis, IR, beamline
Nachgewiesen in Dimensions
Web of Science
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