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Electrolyte Measures to Prevent Polysulfide Shuttle in Lithium‐Sulfur Batteries

Di Donato, Graziano 1; Ates, Tugce 1; Adenusi, Henry; Varzi, Alberto ORCID iD icon 1; Navarra, Maria Assunta ; Passerini, Stefano 1
1 Karlsruher Institut für Technologie (KIT)

Abstract:

Lithium-sulfur (Li−S) batteries are recognized as one of the most promising technologies with the potential to become the next-generation batteries. However, to ensure Li−S batteries reach commercialization, complex challenges remain, among which the tailoring of an appropriate electrolyte is the most important. This review discusses the role of electrolytes in Li−S batteries, focusing on the main issues and solutions for the shuttle mechanism of polysulfides and the instability of the interface with lithium metal. Herein, we present a background on Li−S chemistry followed by the state-of-the-art electrolytes highlighting the different strategies undertaken with liquid and solid electrolytes.


Verlagsausgabe §
DOI: 10.5445/IR/1000146891
Veröffentlicht am 21.10.2022
Originalveröffentlichung
DOI: 10.1002/batt.202200097
Scopus
Zitationen: 11
Web of Science
Zitationen: 16
Dimensions
Zitationen: 20
Cover der Publikation
Zugehörige Institution(en) am KIT Helmholtz-Institut Ulm (HIU)
Publikationstyp Zeitschriftenaufsatz
Publikationsjahr 2022
Sprache Englisch
Identifikator ISSN: 2566-6223
KITopen-ID: 1000146891
HGF-Programm 38.02.01 (POF IV, LK 01) Fundamentals and Materials
Erschienen in Batteries and Supercaps
Verlag John Wiley and Sons
Band 5
Heft 7
Seiten e202200097
Vorab online veröffentlicht am 18.05.2022
Nachgewiesen in Scopus
Web of Science
Dimensions
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