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Precursor region with full phonon softening above the charge-density-wave phase transition in 2H-TaSe$_2$

Weber, Frank ORCID iD icon 1; Shen, Xingchen 1; Heid, Rolf 1; Hott, Roland 1; Haghighirad, Amir-Abbas 1; Salzmann, Björn; Cantarino, Marli dos Reis; Monney, Claude; Said, Ayman H.; Frachet, Mehdi 1; Murphy, Bridget; Rossnagel, Kai; Rosenkranz, Stephan
1 Institut für QuantenMaterialien und Technologien (IQMT), Karlsruher Institut für Technologie (KIT)

Abstract (englisch):

Research on charge-density-wave (CDW) ordered transition-metal dichalcogenides continues to unravel new states of quantum matter correlated to the intertwined lattice and electronic degrees of freedom. Here, we report an inelastic x-ray scattering investigation of the lattice dynamics of the canonical CDW compound 2H-TaSe2 complemented by angle-resolved photoemission spectroscopy and density functional perturbation theory. Our results rule out the formation of a central-peak without full phonon softening for the CDW transition in 2H-TaSe2 and provide evidence for a novel precursor region above the CDW transition temperature TCDW, which is characterized by an overdamped phonon mode and not detectable in our photoemission experiments. Thus, 2H-TaSe2 exhibits structural before electronic static order and emphasizes the important lattice contribution to CDW transitions. Our ab-initio calculations explain the interplay of electron-phonon coupling and Fermi surface topology triggering the CDW phase transition and predict that the CDW soft phonon mode promotes emergent superconductivity near the pressure-driven CDW quantum critical point.


Zugehörige Institution(en) am KIT Institut für QuantenMaterialien und Technologien (IQMT)
Publikationstyp Forschungsdaten
Publikationsdatum 24.10.2023
Erstellungsdatum 18.10.2023
Identifikator DOI: 10.35097/1771
KITopen-ID: 1000163169
Lizenz Creative Commons Namensnennung 4.0 International
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