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Hybridization of lattice and charge order excitations in a superconducting cuprate

Souliou, Sofia-Michaela 1; Ishikawa, Daisuke; Heid, Rolf 1; Bessas, Dimitrios; Kim, Hun-ho; Betto, Davide; Nakata, Suguru; Merz, Michael 1,2; Minola, Matteo; Keimer, Bernhard; Baron, Alfred Q. R. ; Tacon, Matthieu Le ORCID iD icon 1
1 Institut für QuantenMaterialien und Technologien (IQMT), Karlsruher Institut für Technologie (KIT)
2 Karlsruhe Nano Micro Facility (KNMF), Karlsruher Institut für Technologie (KIT)

Abstract:

The ubiquitous tendency of superconducting cuprates to form charge density waves (CDWs) has reignited interest in the nature of their electron-phonon interaction and its role in shaping their phase diagrams. While pronounced dispersion anomalies were reported in several phonon branches, their precise connection to charge order and superconductivity remains unresolved. Here, using high-resolution inelastic x-ray scattering under low temperature and high magnetic field, we uncover a striking phonon renormalization in YBa2Cu3O6+x. It appears along a reciprocal space trajectory connecting the wave vectors of a short-range 2D-CDW, emerging above the superconducting transition, and a long-range 3D-CDW, appearing only when superconductivity is strongly suppressed. The spectral changes are strongest around the wave vector of the 3D-CDW despite the fact that it is absent in our experimental conditions. Our findings challenge conventional phonon self-energy renormalization models, instead support a scenario in which low-energy phonons hybridize with dispersive CDW excitations and provide insights into the interplay between lattice vibrations and electronic correlations in high-temperature superconductors.


Verlagsausgabe §
DOI: 10.5445/IR/1000184390
Veröffentlicht am 01.09.2025
Cover der Publikation
Zugehörige Institution(en) am KIT Institut für QuantenMaterialien und Technologien (IQMT)
Publikationstyp Zeitschriftenaufsatz
Publikationsmonat/-jahr 09.2025
Sprache Englisch
Identifikator ISSN: 2399-3650
KITopen-ID: 1000184390
HGF-Programm 47.11.02 (POF IV, LK 01) Emergent Quantum Phenomena
Erschienen in Communications Physics
Verlag Nature Research
Band 8
Heft 1
Seiten 362
Vorab online veröffentlicht am 01.09.2025
Schlagwörter 032345
Nachgewiesen in Web of Science
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