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Orbital Ordering in the Charge Density Wave Phases of BaNi$_2$(As$_{1-x}$P$_x$)$_2$

Lacmann, Tom ORCID iD icon 1; Eder, Robert 1; Vinograd, Igor 1; Merz, Michael 1,2; Frachet, Mehdi 1; McGuinness, Philippa Helen 1; Kummer, Kurt; Schierle, Enrico; Haghighirad, Amir-Abbas 1; Souliou, Sofia-Michaela 1; Le Tacon, Matthieu ORCID iD icon 1
1 Institut für QuantenMaterialien und Technologien (IQMT), Karlsruher Institut für Technologie (KIT)
2 Karlsruhe Nano Micro Facility (KNMF), Karlsruher Institut für Technologie (KIT)

Abstract:

We use resonant x-ray scattering at the nickel L$_{2;3}$ edges to investigate the interplay between orbital degrees of freedom and charge density waves (CDWs) in the superconductor BaNi$_2$(As$_{1-x}$P$_x$)$_2$. Both the incommensurate and commensurate CDWs in this system exhibit strong resonant enhancement with distinct energy and polarization dependencies, indicative of orbital ordering. Azimuthal-angle-dependent measurements reveal a lowering of the local Ni site symmetry, consistent with monoclinic or lower point group symmetry. The scattering signatures of both CDWs are dominated by contributions from Ni d$_{xz;yz}$ orbitals, with similar orbital character despite their distinct wave vectors. These findings point to a shared orbital-driven formation mechanism and provide new insight into the symmetry breaking and orbital and nematic fluctuations in the high-temperature regime of the superconductor BaNi$_2$(As$_{1-x}$P$_x$)$_2$.


Verlagsausgabe §
DOI: 10.5445/IR/1000189917
Veröffentlicht am 26.01.2026
Cover der Publikation
Zugehörige Institution(en) am KIT Institut für QuantenMaterialien und Technologien (IQMT)
Karlsruhe Nano Micro Facility (KNMF)
Publikationstyp Zeitschriftenaufsatz
Publikationsdatum 23.01.2026
Sprache Englisch
Identifikator ISSN: 0031-9007, 1079-7114
KITopen-ID: 1000189917
HGF-Programm 47.11.02 (POF IV, LK 01) Emergent Quantum Phenomena
Erschienen in Physical Review Letters
Verlag American Physical Society (APS)
Band 136
Heft 3
Seiten Article no: 036504
Nachgewiesen in OpenAlex
Scopus
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