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Radiative neutron capture cross section of $^{242}$Pu measured at n_TOF-EAR1 in the unresolved resonance region up to 600 keV

n_TOF Collaboration; Lerendegui-Marco, J. ; Guerrero, C.; Mendoza, E.; Quesada, J. M.; Eberhardt, K.; Junghans, A. R.; Alcayne, V.; Babiano, V.; Aberle, O.; Andrzejewski, J.; Audouin, L.; Bacak, M.; Balibrea-Correa, J.; Barbagallo, M.; Barros, S.; Bečvář, F.; Bécares, V.; Beinrucker, C.; ... mehr

Abstract:

Accurate neutron capture cross sections are essential for the design and operation of fast reactors using MOX fuels. For $^{242}$Pu, the Nuclear Energy Agency (NEA) recommends 8–12% accuracy in the fast energy region (2–500 keV), compared to the current uncertainty of 35%. Moreover, integral experiments and previous measurements suggest the evaluated $^{242}$Pu(n,$\gamma$) cross section is overestimated, particularly in the JEFF-3.3 library, which shows a 14% overestimation between 1 keV and 1 MeV. Recent measurements from LANSCE reported a 20–30% reduction in the 1–40 keV range relative to evaluations. To solve these discrepancies, the Pu(n,) cross section was measured from 1 to 600 keV at CERN n_TOF-EAR1 facility using a 95(4) mg $^{242}$Pu target, enriched to 99.959%. Gamma rays from neutron capture were detected with an array of C$_6$D$_6$ scintillators and a novel application of the Pulse Height Weighting Technique was employed. The resulting cross section presents a systematic uncertainty between 8 and 12%, reducing the current uncertainties of 35% and achieving the accuracy requested by the NEA. Analysis using FITACS produced average resonance parameters, consistent with the analysis of the resolved resonance region. ... mehr


Verlagsausgabe §
DOI: 10.5445/IR/1000191431
Veröffentlicht am 25.03.2026
Cover der Publikation
Zugehörige Institution(en) am KIT Zukunftscampus (CAMPUS)
Publikationstyp Zeitschriftenaufsatz
Publikationsjahr 2026
Sprache Englisch
Identifikator ISSN: 1434-6001, 1434-601X
KITopen-ID: 1000191431
Erschienen in The European Physical Journal A
Verlag Springer-Verlag
Band 62
Heft 2
Seiten 33
Vorab online veröffentlicht am 20.02.2026
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