Validation of farm-scale methane emissions using nocturnal boundary layer budgets

This study provides the first experimental validation of Swiss agricultural methane emission estimates at the farm scale. We measured CH4 concentrations at a Swiss farmstead during two intensive field campaigns in August 2011 and July 2012 to (1) quantify the source strength of livestock methane emissions using a tethered balloon system and (2) to validate inventory emission estimates via nocturnal boundary layer (NBL) budgets. Field measurements were performed at a distance of 150m from the nearest farm buildings with a tethered balloon system in combination with gradient measurements at eight heights on a 10m tower to better resolve the near-surface concentrations. Vertical profiles of air temperature, relative humidity, CH4 concentration, wind speed, and wind direction showed that the NBL was strongly influenced by local transport processes and by the valley wind system. Methane concentrations showed a pronounced time course, with highest concentrations in the second half of the night. NBL budget flux estimates were obtained via a time–space kriging approach. Main uncertainties of NBL budget flux estimates were associated with nonstationary atmospheric conditions and the estimate of the inversion height zi (top of volume integration). ... mehrThe mean NBL budget fluxes of 1:60$\pm$0:31 μgCH$_{4}$m$^{-2}$ s$^{-1}$ (1:40$\pm$0:50 and 1:66$\pm$0:20 μgCH$_{4}$m$^{-2}$ s$^{-1}$ in 2011 and 2012 respectively) were in good agreement with local inventory estimates based on current livestock number and default emission factors, with 1:29$\pm$0:47 and 1:74$\pm$0:63 μgCH$_{4}$m$^{-2}$ s$^{-1}$ for 2011 and 2012 respectively. This indicates that emission factors used for the national inventory reports are adequate, and we conclude that the NBL budget approach is a useful tool to validate emission inventory estimates.