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Sources and contributions of wood smoke during winter in London: Assessing local and regional influences

Crilley, L.R.; Bloss, W.J.; Yin, J.; Beddows, D.C.S.; Harrison, R.M.; Allan, J.D.; Young, D.E.; Flynn, M.; Williams, P.; Zotter, P.; Prevot, A.S.H.; Heal, M.R.; Barlow, J.F.; Halios, C.H.; Lee, J.D.; Szidat, S.; Mohr, C.

Abstract:
Determining the contribution of wood smoke to air pollution in large cities such as London is becoming increasingly important due to the changing nature of domestic heating in urban areas. During winter, biomass burning emissions have been identified as a major cause of exceedances of European air quality limits. The aim of this work was to quantify the contribution of biomass burning in London to concentrations of PM2:5 and determine whether local emissions or regional contributions were the main source of biomass smoke. To achieve this, a number of biomass burning chemical tracers were analysed at a site within central London and two sites in surrounding rural areas. Concentrations of levoglucosan, elemental carbon (EC), organic carbon (OC) and KC were generally well correlated across the three sites. At all the sites, biomass burning was found to be a source of OC and EC, with the largest contribution of EC from traffic emissions, while for OC the dominant fraction included contributions from secondary organic aerosols, primary biogenic and cooking sources. Source apportionment of the EC and OC was found to give reasonable estima ... mehr

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Verlagsausgabe §
DOI: 10.5445/IR/110104155
Veröffentlicht am 29.10.2018
Originalveröffentlichung
DOI: 10.5194/acp-15-3149-2015
Scopus
Zitationen: 38
Web of Science
Zitationen: 34
Coverbild
Zugehörige Institution(en) am KIT Institut für Meteorologie und Klimaforschung - Atmosphärische Aerosolforschung (IMK-AAF)
Publikationstyp Zeitschriftenaufsatz
Jahr 2015
Sprache Englisch
Identifikator ISSN: 1680-7316, 1680-7324
urn:nbn:de:swb:90-AAA1101041558
KITopen-ID: 110104155
HGF-Programm 12.03.03 (POF III, LK 01)
Erschienen in Atmospheric chemistry and physics
Band 15
Heft 6
Seiten 3149-3171
Nachgewiesen in Scopus
Web of Science
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