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URN: urn:nbn:de:swb:90-424740

Surface Reaction Kinetics for Oxidation and Reforming of H2, CO, and CH4 over Nickel-based Catalysts

Herrera Delgado, Karla

Abstract:
An experimental and kinetic modeling study of H2 and CO oxidation, as well as conversion of methane under oxidative and reforming conditions over nickel-based catalyst is presented. The numerical model is based on a newly developed surface reaction mechanism consisting of 52 elementary-steps reactions with 14 surface and 6 gas-phase species. The mechanism was evaluated against experimental data at varying operating conditions performed in this study and also taken from literature.


Zugehörige Institution(en) am KIT Institut für Technische Chemie und Polymerchemie (ITCP)
Publikationstyp Hochschulschrift
Jahr 2014
Sprache Englisch
Identifikator KITopen ID: 1000042474
Verlag Karlsruhe
Abschlussart Dissertation
Fakultät Fakultät für Chemie und Biowissenschaften (CHEM-BIO)
Institut Institut für Technische Chemie und Polymerchemie (ITCP)
Prüfungsdaten 18.07.2014
Referent/Betreuer Prof. O. Deutschmann
Schlagworte Reaction mechanism, oxidation, reforming, nickel, kinetics
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