Surface Reaction Kinetics for Oxidation and Reforming of H2, CO, and CH4 over Nickel-based Catalysts
Herrera Delgado, Karla
Abstract:
An experimental and kinetic modeling study of H2 and CO oxidation, as well as conversion of methane under oxidative and reforming conditions over nickel-based catalyst is presented. The numerical model is based on a newly developed surface reaction mechanism consisting of 52 elementary-steps reactions with 14 surface and 6 gas-phase species. The mechanism was evaluated against experimental data at varying operating conditions performed in this study and also taken from literature.
| Zugehörige Institution(en) am KIT | Institut für Technische Chemie und Polymerchemie (ITCP) |
| Publikationstyp | Hochschulschrift |
| Publikationsjahr | 2014 |
| Sprache | Englisch |
| Identifikator | urn:nbn:de:swb:90-424740 KITopen-ID: 1000042474 |
| Verlag | Karlsruher Institut für Technologie (KIT) |
| Art der Arbeit | Dissertation |
| Fakultät | Fakultät für Chemie und Biowissenschaften (CHEM-BIO) |
| Institut | Institut für Technische Chemie und Polymerchemie (ITCP) |
| Prüfungsdaten | 18.07.2014 |
| Schlagwörter | Reaction mechanism, oxidation, reforming, nickel, kinetics |
| Nachgewiesen in | OpenAlex |
| Referent/Betreuer | Deutschmann, O. |
