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Enabling Modular Autonomous Feedback-Loops in Materials Science through Hierarchical Experimental Laboratory Automation and Orchestration

Rahmanian, Fuzhan; Flowers, Jackson; Guevarra, Dan; Richter, Matthias; Fichtner, Maximilian; Donnely, Phillip; Gregoire, John M.; Stein, Helge S. ORCID iD icon

Abstract:

Materials acceleration platforms (MAPs) operate on the paradigm of integrating combinatorial synthesis, high-throughput characterization, automatic analysis, and machine learning. Within a MAP, one or multiple autonomous feedback loops may aim to optimize materials for certain functional properties or to generate new insights. The scope of a given experiment campaign is defined by the range of experiment and analysis actions that are integrated into the experiment framework. Herein, the authors present a method for integrating many actions within a hierarchical experimental laboratory automation and orchestration (HELAO) framework. They demonstrate the capability of orchestrating distributed research instruments that can incorporate data from experiments, simulations, and databases. HELAO interfaces laboratory hardware and software distributed across several computers and operating systems for executing experiments, data analysis, provenance tracking, and autonomous planning. Parallelization is an effective approach for accelerating knowledge generation provided that multiple instruments can be effectively coordinated, which the authors demonstrate with parallel electrochemistry experiments orchestrated by HELAO. ... mehr


Verlagsausgabe §
DOI: 10.5445/IR/1000142061
Veröffentlicht am 20.01.2022
Originalveröffentlichung
DOI: 10.1002/admi.202101987
Scopus
Zitationen: 21
Web of Science
Zitationen: 21
Dimensions
Zitationen: 25
Cover der Publikation
Zugehörige Institution(en) am KIT Helmholtz-Institut Ulm (HIU)
Institut für Nanotechnologie (INT)
Institut für Physikalische Chemie (IPC)
Post Lithium Storage (POLiS)
Publikationstyp Zeitschriftenaufsatz
Publikationsjahr 2022
Sprache Englisch
Identifikator ISSN: 2196-7350
KITopen-ID: 1000142061
HGF-Programm 38.02.01 (POF IV, LK 01) Fundamentals and Materials
Erschienen in Advanced Materials Interfaces
Verlag John Wiley and Sons
Band 8
Heft 9
Seiten 2101987
Bemerkung zur Veröffentlichung Special Issue: Advanced Battery Materials and Interfaces — A European Perspective
Vorab online veröffentlicht am 06.01.2022
Nachgewiesen in Web of Science
Dimensions
Scopus
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