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Highly Active Ice‐Nucleating Particles at the Summer North Pole

Porter, Grace C. E.; Adams, Michael P.; Brooks, Ian M.; Ickes, Luisa; Karlsson, Linn; Leck, Caroline; Salter, Matthew E.; Schmale, Julia; Siegel, Karolina; Sikora, Sebastien N. F.; Tarn, Mark D.; Vüllers, Jutta 1; Wernli, Heini; Zieger, Paul; Zinke, Julika; Murray, Benjamin J.
1 Institut für Meteorologie und Klimaforschung – Atmosphärische Spurenstoffe und Fernerkundung (IMK-ASF), Karlsruher Institut für Technologie (KIT)

Abstract:

The amount of ice versus supercooled water in clouds is important for their radiative properties and role in climate feedbacks. Hence, knowledge of the concentration of ice-nucleating particles (INPs) is needed. Generally, the concentrations of INPs are found to be very low in remote marine locations allowing cloud water to persist in a supercooled state. We had expected the concentrations of INPs at the North Pole to be very low given the distance from open ocean and terrestrial sources coupled with effective wet scavenging processes. Here we show that during summer 2018 (August and September) high concentrations of biological INPs (active at >−20°C) were sporadically present at the North Pole. In fact, INP concentrations were sometimes as high as those recorded at mid-latitude locations strongly impacted by highly active biological INPs, in strong contrast to the Southern Ocean. Furthermore, using a balloon borne sampler we demonstrated that INP concentrations were often different at the surface versus higher in the boundary layer where clouds form. Back trajectory analysis suggests strong sources of INPs near the Russian coast, possibly associated with wind-driven sea spray production, whereas the pack ice, open leads, and the marginal ice zone were not sources of highly active INPs. ... mehr


Verlagsausgabe §
DOI: 10.5445/IR/1000145522
Veröffentlicht am 28.04.2022
Originalveröffentlichung
DOI: 10.1029/2021JD036059
Scopus
Zitationen: 26
Web of Science
Zitationen: 25
Dimensions
Zitationen: 37
Cover der Publikation
Zugehörige Institution(en) am KIT Institut für Meteorologie und Klimaforschung – Atmosphärische Spurenstoffe und Fernerkundung (IMK-ASF)
Publikationstyp Zeitschriftenaufsatz
Publikationsdatum 27.03.2022
Sprache Englisch
Identifikator ISSN: 2169-897X, 0148-0227, 2156-2202, 2169-8996
KITopen-ID: 1000145522
HGF-Programm 12.11.26 (POF IV, LK 01) Aerosol-Cloud-Climate-Interaction
Erschienen in Journal of Geophysical Research: Atmospheres
Verlag John Wiley and Sons
Band 127
Heft 6
Seiten e2021JD036059
Vorab online veröffentlicht am 17.03.2022
Nachgewiesen in Scopus
Web of Science
Dimensions
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